Jin, Qinhan and Wu, Wenzhi and Zheng, Zhiren and Yan, Yuxi and Liu, Weilong and Li, Aihua and Yang, Yanqiang and Su, Wenhui (2009) The third-order optical nonlinearity and upconversion luminescence of CdTe quantum dots under femtosecond laser excitation. Journal of Nanoparticle Research, 11 (3). pp. 665-670.
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The aqueous CdTe quantum dots (QDs) were synthesized by the electrostatic reaction method. The optical properties of CdTe QDs were investigated by femtosecond Z-scan and time-resolved luminescence technique in nonresonant spectral region. The nonlinear absorption and refraction are ascribed to two-photon absorption, and time-resolved upconversion photoluminescence produces biexponential decay pattern at infrared femtosecond laser excitation. Upconversion luminescence is composed of a band-edge excitonic state and a photoinduced trapping state. The short-lived band-edge excitonic emission is independent of the detection wavelengths, and long-lived species becomes even longer with the increase of detection wavelengths, which indicates the size dependence of surface excitonic emission.
|Deposited By:||Prof. Alexey Ivanov|
|Deposited On:||16 Mar 2009 09:43|
|Last Modified:||08 May 2009 23:37|
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